Facile fabrication of N-doped heterostructured hybrid particles based on montmorillonite incorporated with g-C3N4 for enhanced hydrogen production by NaBH4 in methanol

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dc.contributor.authorSaka, Cafer
dc.date.accessioned2024-12-24T19:27:01Z
dc.date.available2024-12-24T19:27:01Z
dc.date.issued2024
dc.departmentSiirt Üniversitesi
dc.description.abstractAs an alternative to the currently increasing use of fossil fuels, hydrogen has become very important as a clean energy carrier. Herein, facile fabrication of N doped-heterostructured hybrid particles based montmorillonite (M) incorporated on graphitic carbon nitride (g-C3N4) with calcination and hydrothermal nitric acid activation was performed. The N-doped heterostructured g-C3N4-M hybrid material was used as a metal-free hybrid catalyst for NaBH4 dehydrogenation in methanol for the first time. The hydrogen generation rate (HGR) of 11,200 ml min-1 g-1 in methanol was obtained. XRD, SEM, FTIR, EDS, XPS and nitrogen adsorption/desorption analyses were used to characterize the physicochemical properties of heterostructured composites. Also, the mechanism of catalytic activity was evaluated with the obtained N-doped g-C3N4-M hybrid material.
dc.identifier.doi10.1016/j.diamond.2023.110740
dc.identifier.issn0925-9635
dc.identifier.issn1879-0062
dc.identifier.scopus2-s2.0-85180377027
dc.identifier.scopusqualityQ1
dc.identifier.urihttps://doi.org/10.1016/j.diamond.2023.110740
dc.identifier.urihttps://hdl.handle.net/20.500.12604/6462
dc.identifier.volume142
dc.identifier.wosWOS:001143036000001
dc.identifier.wosqualityQ2
dc.indekslendigikaynakWeb of Science
dc.indekslendigikaynakScopus
dc.language.isoen
dc.publisherElsevier Science Sa
dc.relation.ispartofDiamond and Related Materials
dc.relation.publicationcategoryMakale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanı
dc.rightsinfo:eu-repo/semantics/closedAccess
dc.snmzKA_20241222
dc.subjectGraphitic carbon nitride
dc.subjectMontmorillonite
dc.subjectHybrid material
dc.subjectNitrogen doping
dc.subjectHydrogen generation
dc.titleFacile fabrication of N-doped heterostructured hybrid particles based on montmorillonite incorporated with g-C3N4 for enhanced hydrogen production by NaBH4 in methanol
dc.typeArticle

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